England's middle-order batsman Moeen Ali completed his century on the second morning, his first century away from home and fourth overall.
Ben Stokes went on to score his fourth Test century.
Stokes was finally dismissed for 128 by pacer Umesh Yadav.
India needed to begin well to keep afloat. Openers Murali Vijay (left) and Gautam Gambhir ensured a stable start to India's first innings. India ended the day on 63 for 0.
Gautam Gambhir was unbeaten on 28 at stumps on the second day.
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England's middle-order batsman Moeen Ali completed his century on the second morning, his first century away from home and fourth overall.
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